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Changes in the composition of the northern polar upper stratosphere in February 2009 after a sudden stratospheric warming
Indexado
WoS WOS:000344053400028
DOI 10.1002/2014JD021698
Año 2014
Tipo artículo de investigación

Citas Totales

Autores Afiliación Chile

Instituciones Chile

% Participación
Internacional

Autores
Afiliación Extranjera

Instituciones
Extranjeras


Abstract



Variability in the chemistry of the upper stratosphere/lowermesosphere region has been analyzed focusing on high latitudes during the boreal winter in 2009 characterized by the strong sudden stratospheric warming (SSW) on 24 January. Data from Michelson Interferometer for Passive Atmospheric Sounding aboard Envisat and the Microwave Limb Sounder on Aura have been used to exemplify these changes. Record high (low) values of O-3 and ClO (temperature and HCl) for the winters of 2005-2012, coupled with a simultaneous enhancement of ClONO2, have been observed in February 2009. This suggests that the very low temperatures favor a more effective ozone production and a greater O-3/O ratio. The latter is the main factor controlling active chlorine partitioning. Increases of ClO lead to high ClONO2 concentrations in the upper stratosphere at high latitudes, where its photodissociation rate is smaller. Since this increase of ClONO2 happens at the expense of HCl, the region of high ClONO2 roughly coincides with the region of low HCl. Although this period was characterized by an elevated stratopause event, the investigated region was not influenced by the descent of mesospheric air rich in NOx. Some limited enhancements in NOx at similar to 1 hPa occurred at latitudes greater than 80 degrees N after about 20 February, but they became consistent only in March. Intrusion of midlatitude air mostly occurred between the SSW and early February. Then, the sum of volume mixing ratios of ClONO2 + ClO + HCl remained approximately constant and close to the values of the other years. In contrast, it was up to 0.2 ppbv lower during the SSW period. These atypical chemical conditions occurred also in February 2006, but 2009 stands out for its long-lasting effects, which persisted until late March.

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Disciplinas de Investigación



WOS
Meteorology & Atmospheric Sciences
Scopus
Sin Disciplinas
SciELO
Sin Disciplinas

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Publicaciones WoS (Ediciones: ISSHP, ISTP, AHCI, SSCI, SCI), Scopus, SciELO Chile.

Colaboración Institucional



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Autores - Afiliación



Ord. Autor Género Institución - País
1 Damiani, Alessandro Hombre Universidad de Santiago de Chile - Chile
2 Funke, Bernd Hombre CSIC - España
3 Lopez-Puertas, Manuel Hombre CSIC - España
4 Gardini, Angela Mujer CSIC - España
5 von Clarmann, Thomas Hombre Karlsruhe Inst Technol - Alemania
6 Santee, Michelle L. - CALTECH - Estados Unidos
7 Froidevaux, Lucien - CALTECH - Estados Unidos
8 CORDERO-CARRASCO, RAUL RODRIGO Hombre Universidad de Santiago de Chile - Chile

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Financiamiento



Fuente
FONDECYT
Fondef
NASA
SOUSEI program, MEXT, JAPAN
USACH-DICYT
EC FEDER
Spanish MCINN

Muestra la fuente de financiamiento declarada en la publicación.

Agradecimientos



Agradecimiento
The support of USACH-DICYT, FONDEF (IT13110034), and FONDECYT (1140239) is gratefully acknowledged. A.D. was also supported by the SOUSEI program, MEXT, JAPAN. Work at the Jet Propulsion Laboratory, California Institute of Technology, was done under contract with NASA. The IAA team was supported by the Spanish MCINN under grant AYA2011-23552 and EC FEDER funds. IMK/IAA-generated MIPAS/Envisat data can be obtained by registered users from the data server: http://www.imk-asf.kit.edu/english/308.php. MLS/Aura data are available at the Jet Propulsion Laboratory MLS website: http://mls.jpl.nasa.gov/index.php.

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