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Floquet Engineering of a Diatomic Molecule through a Bichromatic Radiation Field
Indexado
WoS WOS:001184799500001
Scopus SCOPUS_ID:85187690086
DOI 10.1021/ACS.JCTC.3C01277
Año 2024
Tipo artículo de investigación

Citas Totales

Autores Afiliación Chile

Instituciones Chile

% Participación
Internacional

Autores
Afiliación Extranjera

Instituciones
Extranjeras


Abstract



We report on a theoretical study of a Cs-2 molecule illuminated by two lasers and show how this can result in novel quantum dynamics. We reveal that these interactions facilitate the bypass of the non-crossing rule, forming light-induced conical intersections and modifiable avoided crossings. Our findings show how laser field orientation and strength, along with initial phase differences, can control molecular-state transitions, especially on the micromotion scale. We also extensively discuss how the interaction of radiation with matter gives rise to the emergence of potential energy surfaces of hybrids of radiation and molecular states. This research advances a technique for manipulating photoassociation processes in Cs-2 molecules, offering potential new avenues in quantum control.

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Disciplinas de Investigación



WOS
Chemistry, Physical
Physics, Atomic, Molecular & Chemical
Scopus
Sin Disciplinas
SciELO
Sin Disciplinas

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Publicaciones WoS (Ediciones: ISSHP, ISTP, AHCI, SSCI, SCI), Scopus, SciELO Chile.

Colaboración Institucional



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Autores - Afiliación



Ord. Autor Género Institución - País
1 Barriga, Edgar - Universidad de Chile - Chile
2 FOA-TORRES, LUIS EDUARDO FRANCISCO Hombre Universidad de Chile - Chile
3 CARDENAS-CARVAJAL, CESAR ANTONIO Hombre Universidad de Chile - Chile
Centro para el Desarrollo de la Nanociencia y la Nanotecnologia - Chile

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Financiamiento



Fuente
FONDECYT
Fondo Nacional de Desarrollo Científico y Tecnológico
NLHPC
Simons Foundation
Centro para el Desarrollo de la Nanociencia y la Nanotecnologia
Agencia Nacional de Investigación y Desarrollo
EU Horizon 2020 research and innovation program
Center for the Development of Nanosciences and Nanotechnology
Abdus Salam International Center for Theoretical Physics and Simons Foundation
Abdus Salam International Center for Theoretical Physics
Center for the Development of Nanosciences and Nanotechnology, CEDENNA
ANID Chile through the Doctoral National Scholarship
EU Horizon 2020 research and innovation program under Maria-Sklodowska-Curie Grant

Muestra la fuente de financiamiento declarada en la publicación.

Agradecimientos



Agradecimiento
We acknowledge the financial support by FONDECYT through grants 1220366 and 1211038 and by EU Horizon 2020 research and innovation program under Maria-Sklodowska-Curie Grant Agreement 837028 (HYDROTRONICS Project). L.E.F.F.T. also acknowledges the support of The Abdus Salam International Center for Theoretical Physics and Simons Foundation. C.C. acknowledges the support from the Center for the Development of Nanosciences and Nanotechnology, CEDENNA AFB 220001. E.B. acknowledges the support of ANID Chile through the Doctoral National Scholarship No. 21192248. Powered@NLHPC: This research was partially supported by the supercomputing infrastructure of the NLHPC (ECM-02).
We acknowledge the financial support by FONDECYT through grants 1220366 and 1211038 and by EU Horizon 2020 research and innovation program under Maria-Sklodowska-Curie Grant Agreement 837028 (HYDROTRONICS Project). L.E.F.F.T. also acknowledges the support of The Abdus Salam International Center for Theoretical Physics and Simons Foundation. C.C. acknowledges the support from the Center for the Development of Nanosciences and Nanotechnology, CEDENNA AFB 220001. E.B. acknowledges the support of ANID Chile through the Doctoral National Scholarship No. 21192248. Powered@NLHPC: This research was partially supported by the supercomputing infrastructure of the NLHPC (ECM-02).

Muestra la fuente de financiamiento declarada en la publicación.