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Emergence of disordered branching patterns in confined chiral nematic liquid crystals
Indexado
WoS WOS:001025287100001
Scopus SCOPUS_ID:85152176897
DOI 10.1073/PNAS.2221000120
Año 2023
Tipo artículo de investigación

Citas Totales

Autores Afiliación Chile

Instituciones Chile

% Participación
Internacional

Autores
Afiliación Extranjera

Instituciones
Extranjeras


Abstract



Spatial branching processes are ubiquitous in nature, yet the mechanisms that drive their growth may vary significantly from one system to another. In soft matter physics, chiral nematic liquid crystals provide a controlled setting to study the emergence and growth dynamic of disordered branching patterns. Via an appropriate forcing, a cholesteric phase may nucleate in a chiral nematic liquid crystal, which self-organizes into an extended branching pattern. It is known that branching events take place when the rounded tips of cholesteric fingers swell, become unstable, and split into two new cholesteric tips. The origin of this interfacial instability and the mechanisms that drive the large-scale spatial organization of these cholesteric patterns remain unclear. In this work, we investigate experimentally the spatial and temporal organization of thermally driven branching patterns in chiral nematic liquid crystal cells. We describe the observations through a mean-field model and find that chirality is responsible for the creation of fingers, regulates their interactions, and controls the tip-splitting process. Furthermore, we show that the complex dynamics of the cholesteric pattern behaves as a probabilistic process of branching and inhibition of chiral tips that drives the large-scale topological organization. Our theoretical findings are in good agreement with the experimental observations.

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Disciplinas de Investigación



WOS
Multidisciplinary Sciences
Scopus
Sin Disciplinas
SciELO
Sin Disciplinas

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Publicaciones WoS (Ediciones: ISSHP, ISTP, AHCI, SSCI, SCI), Scopus, SciELO Chile.

Colaboración Institucional



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Autores - Afiliación



Ord. Autor Género Institución - País
1 Echeverria-Alar, S. Hombre Universidad de Chile - Chile
2 CLERC-GAVILAN, MARCEL GABRIEL Hombre Universidad de Chile - Chile
3 Bordeu, Ignacio Hombre Universidad de Chile - Chile

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Financiamiento



Fuente
FONDECYT
Universidad de Chile
Fondo Nacional de Desarrollo Científico y Tecnológico
ANID-Millenium Science Initiative Program
ANID by Beca Doctorado Nacional
ANID-Millenium
ANID-Millenium Science Initiative Program-ICN17_012 (MIRO)
Universidad de Chile-VID project

Muestra la fuente de financiamiento declarada en la publicación.

Agradecimientos



Agradecimiento
ACKNOWLEDGMENTS. We acknowledge P.I. Hidalgo and J. Vergara for the synthetization of the cholesteric liquid crystal. M.G.C. thanks for the financial support of ANID-Millenium Science Initiative Program–ICN17_012 (MIRO) and FONDECYT project 1210353. I.B. acknowledges the financial support from FONDECYT project 11230941 and the Universidad de Chile-VID project UI-015/22. We also thank Gregorio González-Cortés for fruitful discussions. Sources of funding: -ANID by Beca Doctorado Nacional 2020-21201376. -ANID-Millenium Science Initiative Program–ICN17_012 (MIRO) -FONDECYT project 1210353.
We acknowledge P.I. Hidalgo and J. Vergara for the synthetization of the cholesteric liquid crystal. M.G.C. thanks for the financial support of ANID-Millenium Science Initiative Program-ICN17_012 (MIRO) and FONDECYT project 1210353. I.B. acknowledges the financial support from FONDECYT project 11230941 and the Universidad de Chile-VID project UI-015/22. We also thank Gregorio Gonzalez-Cortes for fruitful discussions. Sources of funding: -ANID by Beca Doctorado Nacional 2020-21201376.-ANID-Millenium Science Initiative Program-ICN17_012 (MIRO) -FONDECYT project 1210353.

Muestra la fuente de financiamiento declarada en la publicación.