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A simple microswimmer model inspired by the general equation for nonequilibrium reversible-irreversible coupling
Indexado
WoS WOS:000536867500001
Scopus SCOPUS_ID:85102908052
DOI 10.1063/5.0003430
Año 2020
Tipo artículo de investigación

Citas Totales

Autores Afiliación Chile

Instituciones Chile

% Participación
Internacional

Autores
Afiliación Extranjera

Instituciones
Extranjeras


Abstract



A simple mean-field microswimmer model is presented. The model is inspired by the nonequilibrium thermodynamics of multi-component fluids that undergo chemical reactions. These thermodynamics can be rigorously described in the context of the GENERIC (general equation for the nonequilibrium reversible-irreversible coupling) framework. More specifically, this approach was recently applied to non-ideal polymer solutions [T. Indei and J. D. Schieber, J. Chem. Phys. 146, 184902 (2017)]. One of the species of the solution is an unreactive polymer chain represented by the bead-spring model. Using this detailed description as inspiration, we then make several simplifying assumptions to obtain a mean-field model for a Janus microswimmer. The swimmer model considered here consists of a polymer dumbbell in a sea of reactants. One of the beads of the dumbbell is allowed to act as a catalyst for a chemical reaction between the reactants. We show that the mean-squared displacement (MSD) of the center of mass of this Janus dumbbell exhibits ballistic behavior at time scales at which the concentration of the reactant is large. The time scales at which the ballistic behavior is observed in the MSD coincide with the time scales at which the cross-correlation between the swimmer's orientation and the direction of its displacement exhibits a maximum. Since the swimmer model was inspired by the GENERIC framework, it is possible to ensure that the entropy generation is always positive, and therefore, the second law of thermodynamics is obeyed.

Revista



Revista ISSN
Journal Of Chemical Physics 0021-9606

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Disciplinas de Investigación



WOS
Chemistry, Physical
Physics, Atomic, Molecular & Chemical
Scopus
Sin Disciplinas
SciELO
Sin Disciplinas

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Publicaciones WoS (Ediciones: ISSHP, ISTP, AHCI, SSCI, SCI), Scopus, SciELO Chile.

Colaboración Institucional



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Autores - Afiliación



Ord. Autor Género Institución - País
1 Córdoba, Andrés Hombre Universidad de Concepción - Chile
2 Schieber, Jay D. Hombre IIT - Estados Unidos
Illinois Institute of Technology - Estados Unidos
Armour College of Engineering - Estados Unidos
3 Indei, Tsutomu Hombre Hokkaido Univ - Japón
Hokkaido University - Japón

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Financiamiento



Fuente
Fondo Nacional de Desarrollo Científico y Tecnológico
Comisión Nacional de Investigación Científica y Tecnológica
CONICYT under FONDECYT
Chilean National Laboratory for High Performance Computing (NLHPC)

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Agradecimientos



Agradecimiento
A.C. acknowledges financial support from CONICYT under FONDECYT (Grant No. 11170056). This work was completed in part with computational resources provided by the Chilean National Laboratory for High Performance Computing (NLHPC, ECM-02).
A.C. acknowledges financial support from CONICYT under FONDECYT (Grant No. 11170056). This work was completed in part with computational resources provided by the Chilean National Laboratory for High Performance Computing (NLHPC, ECM-02).

Muestra la fuente de financiamiento declarada en la publicación.