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Anthropogenic radionuclides in the water column and a sediment core from the Alboran Sea: application to radiometric dating and reconstruction of historical water column radionuclide concentrations
Indexado
WoS WOS:000259081500006
Scopus SCOPUS_ID:51649091696
DOI 10.1007/S10933-008-9201-Y
Año 2008
Tipo artículo de investigación

Citas Totales

Autores Afiliación Chile

Instituciones Chile

% Participación
Internacional

Autores
Afiliación Extranjera

Instituciones
Extranjeras


Abstract



Global fallout is the main source of anthropogenic radionuclides in the Mediterranean Sea. This work presents Cs-137, Pu239+240 and Am-241 concentrations in the water column in the southwest Alboran Sea, which was sampled in December 1999. A sediment core was taken at 800 m depth in the area (35 degrees 47' N, 04 degrees 48'W). Pb-210, Ra-226, Cs-137 and Pu239+240 specific activities were measured at multiple depths in the core for dating purposes. Cs-137 and Pu239+240 profiles did not show defined peaks that could be used as time markers, and they extended up to depths for which the Pb-210-based constant rate of supply (CRS) dating model provided inconsistent dates. These profiles can be useful to test dating models, understood as particular solutions of a general advection-diffusion problem, if the time series of radionuclide inputs into the sediment is provided. Thus, historical records of depth-averaged Cs-137 and Pu239+240 concentrations in water, and their corresponding fluxes into the sediment, were reconstructed. A simple water-column model was used for this purpose, involving atmospheric fallout, measured distribution coefficient (k(d)) values, and a first-estimate of sedimentation rates. A dating model of constant mixing with constant sedimentation rate was applied successfully to three independent records (unsupported Pb-210, Cs-137 and Pu239+240), and provided the objective determination of mixing parameters and mass sedimentation rate. These results provide some insight into the fate of atmospheric inputs to this marine environment and, particularly, into the contribution from the Chernobyl accident.

Revista



Revista ISSN
Journal Of Paleolimnology 0921-2728

Métricas Externas



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Disciplinas de Investigación



WOS
Geosciences, Multidisciplinary
Environmental Sciences
Limnology
Scopus
Sin Disciplinas
SciELO
Sin Disciplinas

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Publicaciones WoS (Ediciones: ISSHP, ISTP, AHCI, SSCI, SCI), Scopus, SciELO Chile.

Colaboración Institucional



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Autores - Afiliación



Ord. Autor Género Institución - País
1 Laissaoui, A. - Ctr Natl Energie Sci & Tech Nucl - Marruecos
National Energy Center of Nuclear Science and Technology - Marruecos
2 Benmansour, Moncef Hombre Ctr Natl Energie Sci & Tech Nucl - Marruecos
National Energy Center of Nuclear Science and Technology - Marruecos
3 Ziad, N. - Ctr Natl Energie Sci & Tech Nucl - Marruecos
National Energy Center of Nuclear Science and Technology - Marruecos
4 Ibn Majah, M. - Ctr Natl Energie Sci & Tech Nucl - Marruecos
National Energy Center of Nuclear Science and Technology - Marruecos
5 Abril, J. M. - Universidad de Sevilla - España
University of Seville - España
Univ Seville - España
6 MULSOW-FLORES, SANDOR GUILLERMO - Universidad Austral de Chile - Chile

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Financiamiento



Fuente
IAEA
International Atomic Energy Agency

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Agradecimientos



Agradecimiento
This work was supported by IAEA under the Regional Project RAF/7/004. The authors acknowledge the support provided by IAEA-Marine Environment Laboratory of Monaco for the sampling cruise. They also thank colleagues from INRH for their assistance during sampling.
Acknowledgements This work was supported by IAEA under the Regional Project RAF/7/004. The authors acknowledge the support provided by IAEA-Marine Environment Laboratory of Monaco for the sampling cruise. They also thank colleagues from INRH for their assistance during sampling.

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