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| DOI | 10.1021/NN900909Q | ||||
| Año | 2009 | ||||
| Tipo | artículo de investigación |
Citas Totales
Autores Afiliación Chile
Instituciones Chile
% Participación
Internacional
Autores
Afiliación Extranjera
Instituciones
Extranjeras
To date, no large-scale preparative method for arrays of nanotube enables the experimentalist to arbitrarily define changes in the tubes' diameter along their length. To this goal, we start with anodic alumina substrates displaying controlled modulations in pore diameter obtained by alternating "mild" and "hard" electrochemical etching conditions. We then utilize atomic layer deposition (ALD) to coat the internal pore walls with conformal layers of an oxide. Ferromagnetic Fe3O4 tubes of 10 nm wall thickness and 10-30 mu m in length are thus prepared, which replicate the modulated silhouette of the template. Their magnetic properties strongly depend on the presence of diameter modulations. Introducing one or several very short segments of large diameter (150 nm) into an otherwise thin tube (70 nm diameter) brings its initially large coercive field down to a value close to the case of a homogeneously thick tube. Theoretical modeling emphasizes the major influence of the magnetostatic interactions between neighboring tubes. They are enhanced locally at the sites of diameter modulations, which directly translates into a reduction in coercive field.
| Ord. | Autor | Género | Institución - País |
|---|---|---|---|
| 1 | Pitzschel, Kristina | Mujer |
UNIV HAMBURG - Alemania
Universität Hamburg - Alemania |
| 2 | Montero-Moreno, Josep M. | Hombre |
UNIV HAMBURG - Alemania
Univ Barcelona - España Universität Hamburg - Alemania Universitat de Barcelona - España |
| 3 | ESCRIG-MURUA, JUAN | Hombre |
Universidad de Santiago de Chile - Chile
|
| 4 | Albrecht, Ole | - |
UNIV HAMBURG - Alemania
Universität Hamburg - Alemania |
| 5 | Nielsch, K. | Hombre |
UNIV HAMBURG - Alemania
Universität Hamburg - Alemania |
| 6 | Bachmann, Julien | Hombre |
UNIV HAMBURG - Alemania
Universität Hamburg - Alemania |
| Fuente |
|---|
| FONDECYT |
| Generalitat de Catalunya |
| Millennium Science Nucleus Basic and Applied Magnetism |
| German Research Council (DFG) |
| Fans Social Europeu |
| German Ministry of Education and ResearchFKZ03X5519 |
| Agradecimiento |
|---|
| We thank D. Gorlitz for insightful discussions and R. Meissner for crucial technical assistance. This work was supported by the German Research Council (DFG) in the framework of the Sondeforschungsbereich SFB668 tismus vom Einzelatorn zur Nanostruktur' and by the German Ministry of Education and Research (BMBF FKZ03X5519). J.M.M. acknowledges the Comissionat per a Universitats i Recerca from the Departament d'Innovaco, Universitats i Empresa from Generalitat de Catalunya, and the Fans Social Europeu for financial support. J.E. acknowledges the "Millennium Science Nucleus Basic and Applied Magnetism" (project P06-022F) and Fondecyt (project 11070010). |