Spatially-resolved maps of mid-IR tropospheric aerosol opacity revealed a well-defined lane of depleted aerosols around the GRS periphery, and a correlation with visibly-dark jovian clouds and bright 4.8-mu m emission. Ammonia showed a similar but broader ring of depletion encircling the GRS. This narrow lane of subsidence keeps red aerosols physically separate from white aerosols external to the GRS. The visibility of the 4.8-mu m bright periphery varies with the mid-IR aerosol opacity of the upper troposphere. Compositional maps of ammonia, phosphine and para-H(2) within the GRS interior all exhibit north-south asymmetries, with evidence for higher concentrations north of the warm central core and the strongest depletions in a symmetric arc near the southern periphery. Small-scale enhancements in temperature. NH(3) and aerosol opacity associated with localized convection are observed within the generally-warm and aerosol-free South Equatorial Belt (SEB) northwest of the GRS. The extent of 4.8-mu m emission from the SEB varied as a part of the 2007 'global upheaval,' though changes during this period were restricted to pressures greater than 500 mbar. Finally, a region of enhanced temperatures extended southwest of the GRS during the survey, restricted to the 100-400 mbar range and with no counterpart in visible imaging or compositional mapping. The warm airmass was perturbed by frequent encounters with the cold airmass of Oval BA, but no internal thermal or compositional effects were noted in either vortex during the close encounters. (C) 2010 Elsevier Inc. All rights reserved.